Direkt zum Inhalt

Schlauderer, Stefan ; Lange, Christoph ; Baierl, Sebastian ; Ebnet, Thomas ; Schmid, Christoph P. ; Valovcin, D. C. ; Zvezdin, A. K. ; Kimel, A. V. ; Mikhaylovskiy, R. V. ; Huber, Rupert

Temporal and spectral fingerprints of ultrafast all-coherent spin switching

Schlauderer, Stefan, Lange, Christoph, Baierl, Sebastian, Ebnet, Thomas, Schmid, Christoph P., Valovcin, D. C., Zvezdin, A. K., Kimel, A. V. , Mikhaylovskiy, R. V. und Huber, Rupert (2019) Temporal and spectral fingerprints of ultrafast all-coherent spin switching. Nature 569, S. 383-387.

Veröffentlichungsdatum dieses Volltextes: 18 Nov 2019 07:30
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.41037


Zusammenfassung

Future information technology demands ever-faster, low-loss quantum control. Intense light fields have facilitated milestones along this way, including the induction of novel states of matter(1-3), ballistic acceleration of electrons(4-7) and coherent flipping of the valley pseudospin(8). These dynamics leave unique 'fingerprints', such as characteristic bandgaps or high-order harmonic radiation. ...

Future information technology demands ever-faster, low-loss quantum control. Intense light fields have facilitated milestones along this way, including the induction of novel states of matter(1-3), ballistic acceleration of electrons(4-7) and coherent flipping of the valley pseudospin(8). These dynamics leave unique 'fingerprints', such as characteristic bandgaps or high-order harmonic radiation. The fastest and least dissipative way of switching the technologically most important quantum attribute-the spin-between two states separated by a potential barrier is to trigger an all-coherent precession. Experimental and theoretical studies with picosecond electric and magnetic fields have suggested this possibility(9-11), yet observing the actual spin dynamics has remained out of reach. Here we show that terahertz electromagnetic pulses allow coherent steering of spins over a potential barrier, and we report the corresponding temporal and spectral fingerprints. This goal is achieved by coupling spins in antiferromagnetic TmFeO3 (thulium orthoferrite) with the locally enhanced terahertz electric field of custom-tailored antennas. Within their duration of one picosecond, the intense terahertz pulses abruptly change the magnetic anisotropy and trigger a large-amplitude ballistic spin motion. A characteristic phase flip, an asymmetric splitting of the collective spin resonance and a long-lived offset of the Faraday signal are hallmarks of coherent spin switching into adjacent potential minima, in agreement with numerical simulations. The switchable states can be selected by an external magnetic bias. The low dissipation and the antenna's subwavelength spatial definition could facilitate scalable spin devices operating at terahertz rates.



Beteiligte Einrichtungen


Verknüpfung von Datensätzen

Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNature
Verlag:Nature
Ort der Veröffentlichung:LONDON
Band:569
Seitenbereich:S. 383-387
Datum15 Mai 2019
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1038/s41586-019-1174-7DOI
Stichwörter / KeywordsDRIVEN; DYNAMICS;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-410371
Dokumenten-ID41037

Bibliographische Daten exportieren

Nur für Besitzer und Autoren: Kontrollseite des Eintrags

nach oben