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Dirnberger, Florian ; Abujetas, D. R. ; König, J. ; Forsch, M. ; Koller, T. ; Gronwald, Imke ; Lange, Christoph ; Huber, Rupert ; Schüller, Christian ; Korn, Tobias ; Sánchez-Gil, J. A. ; Bougeard, Dominique

Tuning spontaneous emission through waveguide cavity effects in semiconductor nanowires

Dirnberger, Florian, Abujetas, D. R., König, J., Forsch, M., Koller, T., Gronwald, Imke, Lange, Christoph, Huber, Rupert , Schüller, Christian, Korn, Tobias , Sánchez-Gil, J. A. and Bougeard, Dominique (2019) Tuning spontaneous emission through waveguide cavity effects in semiconductor nanowires. Nano Letters 19, pp. 7287-7292.

Date of publication of this fulltext: 18 Nov 2019 07:08
Article
DOI to cite this document: 10.5283/epub.41040


Abstract

The ability to tailor waveguide cavities and couple them with quantum emitters has developed a realm of nanophotonics encompassing, for example, highly efficient single photon generation or the control of giant photon nonlinearities. Opening new grounds by pushing the interaction of the waveguide cavity and integrated emitters further into the deep subwavelength regime, however, has been ...

The ability to tailor waveguide cavities and couple them with quantum emitters has developed a realm of nanophotonics encompassing, for example, highly efficient single photon generation or the control of giant photon nonlinearities. Opening new grounds by pushing the interaction of the waveguide cavity and integrated emitters further into the deep subwavelength regime, however, has been complicated by nonradiative losses due to the increasing importance of surface defects when decreasing cavity dimensions. Here, we show efficient suppression of nonradiative recombination for thin waveguide cavities using core-shell semiconductor nanowires. We experimentally reveal the advantages of such nanowires, which host mobile emitters, that is, free excitons, in a one-dimensional (1D) waveguide, highlighting the resulting potential for tunable, active, nanophotonic devices. In our experiment, controlling the nanowire waveguide diameter tunes the luminescence lifetime of excitons in the nanowires across 2 orders of magnitude up to 80 ns. At the smallest wire diameters, we show that this luminescence lifetime can be manipulated by engineering the dielectric environment of the nanowires. Exploiting this unique handle on the spontaneous emission of mobile emitters, we demonstrate an all-dielectric spatial control of the mobile emitters along the axis of the 1D nanowire waveguide.



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Details

Item typeArticle
Journal or Publication TitleNano Letters
Publisher:AMER CHEMICAL SOC
Open Access Type:Due to SHERPA/RoMEO
Place of Publication:WASHINGTON
Volume:19
Page Range:pp. 7287-7292
Date16 September 2019
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Dominique Bougeard
Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Dominique Bougeard
Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group Christian Schüller
Identification Number
ValueType
10.1021/acs.nanolett.9b02883DOI
KeywordsSINGLE-NANOWIRE; GAAS NANOWIRES; CARRIER LIFETIME; N-TYPE; ENHANCEMENT; SURFACE; MODES; INP; Semiconductor nanowire; luminescence lifetime; tunable spontaneous emission; photonic waveguide cavity; free excitons; subwavelength nanophotonics
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-410402
Item ID41040

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