Direkt zum Inhalt

Zollner, Klaus ; Faria Junior, Paulo E. ; Fabian, Jaroslav

Proximity exchange effects in MoSe2 and WSe2 heterostructures with CrI3: Twist angle, layer, and gate dependence

Zollner, Klaus, Faria Junior, Paulo E. und Fabian, Jaroslav (2019) Proximity exchange effects in MoSe2 and WSe2 heterostructures with CrI3: Twist angle, layer, and gate dependence. Phys. Rev. B 100, 085128.

Veröffentlichungsdatum dieses Volltextes: 18 Dez 2019 13:58
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.41296


Zusammenfassung

Proximity effects in two-dimensional (2D) van der Waals heterostructures offer controllable ways to tailor the electronic band structure of adjacent materials. Proximity exchange in particular is important for making materials magnetic without hosting magnetic ions. Such synthetic magnets could be used for studying magnetotransport in high-mobility 2D materials, or magneto-optics in highly ...

Proximity effects in two-dimensional (2D) van der Waals heterostructures offer controllable ways to tailor the electronic band structure of adjacent materials. Proximity exchange in particular is important for making materials magnetic without hosting magnetic ions. Such synthetic magnets could be used for studying magnetotransport in high-mobility 2D materials, or magneto-optics in highly absorptive nominally nonmagnetic semiconductors. Using first-principles calculations, we show that the proximity exchange in monolayer MoSe2 and WSe2 due to ferromagnetic monolayer CrI3 can be tuned (even qualitatively) by twisting and gating. Remarkably, the proximity exchange remains the same when using antiferromagnetic CrI3 bilayer, paving the way for optical and electrical detection of layered antiferromagnets. Interestingly, the proximity exchange is opposite to the exchange of the adjacent antiferromagnetic layer. Finally, we show that the proximity exchange is confined to the layer adjacent to CrI3, and that adding a separating hBN barrier drastically reduces the proximity effect. We complement our ab initio results with tight-binding modeling and solve the Bethe-Salpeter equation to provide experimentally verifiable optical signatures (in the exciton spectra) of the proximity exchange effects.



Beteiligte Einrichtungen


Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftPhys. Rev. B
Verlag:AMER PHYSICAL SOC
Ort der Veröffentlichung:COLLEGE PK
Band:100
Seitenbereich:085128
DatumAugust 2019
InstitutionenPhysik > Institut für Theoretische Physik
Physik > Institut für Theoretische Physik > Lehrstuhl Professor Richter > Arbeitsgruppe Jaroslav Fabian
Identifikationsnummer
WertTyp
10.1103/PhysRevB.100.085128DOI
Stichwörter / KeywordsVALLEY POLARIZATION; INTRINSIC FERROMAGNETISM; ELECTRONIC-STRUCTURES; CRYSTAL-STRUCTURE; MONOLAYER MOTE2; GRAPHENE; PHOTOLUMINESCENCE; EXCITATIONS; MAGNETISM;
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-412963
Dokumenten-ID41296

Bibliographische Daten exportieren

Nur für Besitzer und Autoren: Kontrollseite des Eintrags

nach oben