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Zollner, Klaus ; Faria Junior, Paulo E. ; Fabian, Jaroslav

Proximity exchange effects in MoSe2 and WSe2 heterostructures with CrI3: Twist angle, layer, and gate dependence

Zollner, Klaus, Faria Junior, Paulo E. and Fabian, Jaroslav (2019) Proximity exchange effects in MoSe2 and WSe2 heterostructures with CrI3: Twist angle, layer, and gate dependence. Phys. Rev. B 100, 085128.

Date of publication of this fulltext: 18 Dec 2019 13:58
Article
DOI to cite this document: 10.5283/epub.41296


Abstract

Proximity effects in two-dimensional (2D) van der Waals heterostructures offer controllable ways to tailor the electronic band structure of adjacent materials. Proximity exchange in particular is important for making materials magnetic without hosting magnetic ions. Such synthetic magnets could be used for studying magnetotransport in high-mobility 2D materials, or magneto-optics in highly ...

Proximity effects in two-dimensional (2D) van der Waals heterostructures offer controllable ways to tailor the electronic band structure of adjacent materials. Proximity exchange in particular is important for making materials magnetic without hosting magnetic ions. Such synthetic magnets could be used for studying magnetotransport in high-mobility 2D materials, or magneto-optics in highly absorptive nominally nonmagnetic semiconductors. Using first-principles calculations, we show that the proximity exchange in monolayer MoSe2 and WSe2 due to ferromagnetic monolayer CrI3 can be tuned (even qualitatively) by twisting and gating. Remarkably, the proximity exchange remains the same when using antiferromagnetic CrI3 bilayer, paving the way for optical and electrical detection of layered antiferromagnets. Interestingly, the proximity exchange is opposite to the exchange of the adjacent antiferromagnetic layer. Finally, we show that the proximity exchange is confined to the layer adjacent to CrI3, and that adding a separating hBN barrier drastically reduces the proximity effect. We complement our ab initio results with tight-binding modeling and solve the Bethe-Salpeter equation to provide experimentally verifiable optical signatures (in the exciton spectra) of the proximity exchange effects.



Involved Institutions


Details

Item typeArticle
Journal or Publication TitlePhys. Rev. B
Publisher:AMER PHYSICAL SOC
Place of Publication:COLLEGE PK
Volume:100
Page Range:085128
DateAugust 2019
InstitutionsPhysics > Institute of Theroretical Physics
Physics > Institute of Theroretical Physics > Chair Professor Richter > Group Jaroslav Fabian
Identification Number
ValueType
10.1103/PhysRevB.100.085128DOI
KeywordsVALLEY POLARIZATION; INTRINSIC FERROMAGNETISM; ELECTRONIC-STRUCTURES; CRYSTAL-STRUCTURE; MONOLAYER MOTE2; GRAPHENE; PHOTOLUMINESCENCE; EXCITATIONS; MAGNETISM;
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-412963
Item ID41296

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