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Mooshammer, Fabian ; Huber, Markus A. ; Sandner, Fabian ; Plankl, Markus ; Zizlsperger, Martin ; Huber, Rupert

Quantifying nanoscale electromagnetic fields in near-field microscopy by Fourier demodulation analysis

Mooshammer, Fabian , Huber, Markus A., Sandner, Fabian, Plankl, Markus, Zizlsperger, Martin und Huber, Rupert (2020) Quantifying nanoscale electromagnetic fields in near-field microscopy by Fourier demodulation analysis. ACS Photonics.

Veröffentlichungsdatum dieses Volltextes: 13 Feb 2020 08:34
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.41573


Zusammenfassung

Confining light to sharp metal tips has become a versatile technique to study optical and electronic properties far below the diffraction limit. Particularly near-field microscopy in the mid-infrared spectral range has found a variety of applications in probing nanostructures and their dynamics. Yet, the ongoing quest for ultimately high spatial resolution down to the single-nanometer regime and ...

Confining light to sharp metal tips has become a versatile technique to study optical and electronic properties far below the diffraction limit. Particularly near-field microscopy in the mid-infrared spectral range has found a variety of applications in probing nanostructures and their dynamics. Yet, the ongoing quest for ultimately high spatial resolution down to the single-nanometer regime and quantitative three-dimensional nano-tomography depends vitally on a precise knowledge of the spatial distribution of the near fields emerging from the probe. Here, we perform finite element simulations of a tip with realistic geometry oscillating above a dielectric sample. By introducing a novel Fourier demodulation analysis of the electric field at each point in space, we reliably quantify the distribution of the near fields above and within the sample. Besides inferring the lateral field extension, which can be smaller than the tip radius of curvature, we also quantify the probing volume within the sample. Finally, we visualize the scattering process into the far field at a given demodulation order, for the first time, and shed light onto the nanoscale distribution of the near fields, and its evolution as the tip-sample distance is varied. Our work represents a crucial step in understanding and tailoring the spatial distribution of evanescent fields in optical nanoscopy.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftACS Photonics
Verlag:AMER CHEMICAL SOC
Ort der Veröffentlichung:WASHINGTON
Datum22 Januar 2020
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik
Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1021/acsphotonics.9b01533DOI
Stichwörter / KeywordsANALYTICAL-MODEL; SPECTROSCOPY; ULTRAFAST; POLARITONS; ABSORPTION; NANOWIRES; PROBES; TIP; scattering-type SNOM; mid-infrared; nanoscopy; tomography; finite element method; demodulated fields
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
Dokumenten-ID41573

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