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Mooshammer, Fabian ; Huber, Markus A. ; Sandner, Fabian ; Plankl, Markus ; Zizlsperger, Martin ; Huber, Rupert

Data archive of "Quantifying Nanoscale Electromagnetic Fields in Near-Field Microscopy by Fourier Demodulation Analysis"

Dataset

Mooshammer, Fabian , Huber, Markus A., Sandner, Fabian, Plankl, Markus, Zizlsperger, Martin and Huber, Rupert (2020) Data archive of "Quantifying Nanoscale Electromagnetic Fields in Near-Field Microscopy by Fourier Demodulation Analysis". [Dataset]

DOI to cite this document: 10.5283/epub.43818


Abstract

Confining light to sharp metal tips has become a versatile technique to study optical and electronic properties far below the diffraction limit. Particularly near-field microscopy in the mid-infrared spectral range has found a variety of applications in probing nanostructures and their dynamics. Yet, the ongoing quest for ultimately high spatial resolution down to the single-nanometer regime and ...

Confining light to sharp metal tips has become a versatile technique to study optical and electronic properties far below the diffraction limit. Particularly near-field microscopy in the mid-infrared spectral range has found a variety of applications in probing nanostructures and their dynamics. Yet, the ongoing quest for ultimately high spatial resolution down to the single-nanometer regime and quantitative three-dimensional nano-tomography depends vitally on a precise knowledge of the spatial distribution of the near fields emerging from the probe. Here, we perform finite element simulations of a tip with realistic geometry oscillating above a dielectric sample. By introducing a novel Fourier demodulation analysis of the electric field at each point in space, we reliably quantify the distribution of the near fields above and within the sample. Besides inferring the lateral field extension, which can be smaller than the tip radius of curvature, we also quantify the probing volume within the sample. Finally, we visualize the scattering process into the far field at a given demodulation order, for the first time, and shed light onto the nanoscale distribution of the near fields, and its evolution as the tip-sample distance is varied. Our work represents a crucial step in understanding and tailoring the spatial distribution of evanescent fields in optical nanoscopy.



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Details

Item typeDataset
Journal or Publication TitleACS Photonics
PublisherAMER CHEMICAL SOC
Place of PublicationWASHINGTON
Volume7
Number of Issue or Book Chapter2
Page Rangepp. 344-351
Date2020
Date of publication28 Sep 2020 07:18
InstitutionsPhysics > Institute of Experimental and Applied Physics
Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Identification Number
ValueType
10.1021/acsphotonics.9b01533DOI
KeywordsANALYTICAL-MODEL; SPECTROSCOPY; ULTRAFAST; POLARITONS; ABSORPTION; NANOWIRES; PROBES; TIP; scattering-type SNOM; mid-infrared; nanoscopy; tomography; finite element method; demodulated fields
Dewey Decimal Classification500 Science > 530 Physics
StatusUnpublished
RefereedNo, this document will not be refereed
Created at the University of RegensburgYes
Item ID43818

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