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Asymmetric nucleophilic dearomatization of diazarenes by anion-binding catalysis

Fischer, Theresa ; Bamberger, Julia ; Mancheño, Olga García


The first anion-binding organocatalyzed enantioselective Reissert-type dearomatization of diazarenes has been developed. This reaction represents a synthetic challenge since diazarenes have various reactive sites. The use of a chiral tetrakistriazole as a C-H-based hydrogen-donor catalyst allowed the straightforward highly regio- and enantioselective synthesis of a variety of chiral diazaheterocycles.

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