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Thermally Tunable Dual Emission of the d8–d8Dimer [Pt2(μ-P2O5(BF2)2)4]4–

Hofbeck, Thomas ; Lam, Yan Choi ; Kalbáč, Martin ; Záliš, Stanislav ; Vlček, Antonín ; Yersin, Hartmut


High-resolution fluorescence, phosphorescence, as well as related excitation spectra, and, in particular, the emission decay behavior of solid [Bu4N](4)[Pt-2(mu-P2O5(BF2)(2))(4)], abbreviated Pt(pop-BF2), have been investigated over a wide temperature range, 1.3-310 K. We focus on the lowest excited states that result from d sigma*p sigma (Sd(z)(2)-6p(z)) excitations, i.e., the singlet state S-1 ...


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