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A Cyclometalated Ruthenium-NHC Precatalyst for the Asymmetric Hydrogenation of (Hetero)arenes and Its Activation Pathway

Paul, Daniel ; Beiring, Bernhard ; Plois, Markus ; Ortega, Nuria ; Kock, Slawomir ; Schlüns, Danny ; Neugebauer, Johannes ; Wolf, Robert ; Glorius, Frank


This study describes the structural investigation of a highly versatile ruthenium-NHC (N-heterocyclic carbene) catalyst complex, which has been established for the asymmetric hydrogenation of various aromatic compounds. A complex containing an unusual doubly deprotonated NHC ligand was isolated and identified as the precatalyst to this complex. When its subsequent reactivity was monitored, two ...


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