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Photocatalytic Reductive Radical‑Polar Crossover for a
Base‑Free Corey‑Seebach Reaction

Donabauer, Karsten ; Murugesan, Kathiravan ; Rozman, Urša ; Crespi, Stefano ; König, Burkhard



Abstract

A metal-free generation of carbanion nucleophiles is of prime importance in organic synthesis. Herein we report a photocatalytic approach to the Corey-Seebach reaction. The presented method operates under mild redox-neutral and base-free conditions giving the desired product with high functional group tolerance. The reaction is enabled by the combination of photo- and hydrogen atom transfer ...

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