Direkt zum Inhalt

Raab, Jürgen ; Mezzapesa, Francesco P. ; Viti, L. ; Dessmann, Nils ; Diebel, Laura K. ; Li, Lianhe ; Davies, A. Giles ; Linfield, Edmund H. ; Lange, Christoph ; Huber, Rupert ; Vitiello, Miriam S.

Ultrafast terahertz saturable absorbers using tailored intersubband polaritons

Raab, Jürgen, Mezzapesa, Francesco P., Viti, L., Dessmann, Nils, Diebel, Laura K., Li, Lianhe , Davies, A. Giles , Linfield, Edmund H. , Lange, Christoph , Huber, Rupert und Vitiello, Miriam S. (2020) Ultrafast terahertz saturable absorbers using tailored intersubband polaritons. Nature Communications 11 (4290).

Veröffentlichungsdatum dieses Volltextes: 25 Sep 2020 06:55
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.43760


Zusammenfassung

Semiconductor heterostructures have enabled a great variety of applications ranging from GHz electronics to photonic quantum devices. While nonlinearities play a central role for cutting-edge functionality, they require strong field amplitudes owing to the weak light-matter coupling of electronic resonances of naturally occurring materials. Here, we ultrastrongly couple intersubband transitions ...

Semiconductor heterostructures have enabled a great variety of applications ranging from GHz electronics to photonic quantum devices. While nonlinearities play a central role for cutting-edge functionality, they require strong field amplitudes owing to the weak light-matter coupling of electronic resonances of naturally occurring materials. Here, we ultrastrongly couple intersubband transitions of semiconductor quantum wells to the photonic mode of a metallic cavity in order to custom-tailor the population and polarization dynamics of intersubband cavity polaritons in the saturation regime. Two-dimensional THz spectroscopy reveals strong subcycle nonlinearities including six-wave mixing and a collapse of light-matter coupling within 900fs. This collapse bleaches the absorption, at a peak intensity one order of magnitude lower than previous all-integrated approaches and well achievable by state-of-the-art QCLs, as demonstrated by a saturation of the structure under cw-excitation. We complement our data by a quantitative theory. Our results highlight a path towards passively mode-locked QCLs based on polaritonic saturable absorbers in a monolithic single-chip design. Structures that can enhance the capabilities of quantum cascade lasers are highly sought after to improve their practicality for a range of applications. Here the authors demonstrate such a structure in a saturable absorber that takes advantage of intersubband polaritons in the terahertz range and study coherent nonlinear dynamics in the system.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNature Communications
Verlag:Nature
Ort der Veröffentlichung:LONDON
Band:11
Nummer des Zeitschriftenheftes oder des Kapitels:4290
Datum27 August 2020
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1038/s41467-020-18004-8DOI
Stichwörter / KeywordsQUANTUM CASCADE LASERS; PULSES; GENERATION; ABSORPTION; LIGHT;
Dewey-Dezimal-Klassifikation600 Technik, Medizin, angewandte Wissenschaften > 610 Medizin
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-437600
Dokumenten-ID43760

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