| Download ( PDF | 1MB) |
Ultrafast terahertz saturable absorbers using tailored intersubband polaritons
Raab, Jürgen, Mezzapesa, Francesco P., Viti, L., Dessmann, Nils, Diebel, Laura K., Li, Lianhe
, Davies, A. Giles
, Linfield, Edmund H.
, Lange, Christoph
, Huber, Rupert und Vitiello, Miriam S.
(2020)
Ultrafast terahertz saturable absorbers using tailored intersubband polaritons.
Nature Communications 11 (4290).
Veröffentlichungsdatum dieses Volltextes: 25 Sep 2020 06:55
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.43760
Zusammenfassung
Semiconductor heterostructures have enabled a great variety of applications ranging from GHz electronics to photonic quantum devices. While nonlinearities play a central role for cutting-edge functionality, they require strong field amplitudes owing to the weak light-matter coupling of electronic resonances of naturally occurring materials. Here, we ultrastrongly couple intersubband transitions ...
Semiconductor heterostructures have enabled a great variety of applications ranging from GHz electronics to photonic quantum devices. While nonlinearities play a central role for cutting-edge functionality, they require strong field amplitudes owing to the weak light-matter coupling of electronic resonances of naturally occurring materials. Here, we ultrastrongly couple intersubband transitions of semiconductor quantum wells to the photonic mode of a metallic cavity in order to custom-tailor the population and polarization dynamics of intersubband cavity polaritons in the saturation regime. Two-dimensional THz spectroscopy reveals strong subcycle nonlinearities including six-wave mixing and a collapse of light-matter coupling within 900fs. This collapse bleaches the absorption, at a peak intensity one order of magnitude lower than previous all-integrated approaches and well achievable by state-of-the-art QCLs, as demonstrated by a saturation of the structure under cw-excitation. We complement our data by a quantitative theory. Our results highlight a path towards passively mode-locked QCLs based on polaritonic saturable absorbers in a monolithic single-chip design. Structures that can enhance the capabilities of quantum cascade lasers are highly sought after to improve their practicality for a range of applications. Here the authors demonstrate such a structure in a saturable absorber that takes advantage of intersubband polaritons in the terahertz range and study coherent nonlinear dynamics in the system.
Alternative Links zum Volltext
Beteiligte Einrichtungen
Details
| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Nature Communications | ||||
| Verlag: | Nature | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | LONDON | ||||
| Band: | 11 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 4290 | ||||
| Datum | 27 August 2020 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | QUANTUM CASCADE LASERS; PULSES; GENERATION; ABSORPTION; LIGHT; | ||||
| Dewey-Dezimal-Klassifikation | 600 Technik, Medizin, angewandte Wissenschaften > 610 Medizin | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Zum Teil | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-437600 | ||||
| Dokumenten-ID | 43760 |
Downloadstatistik
Downloadstatistik