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Photocatalyzed Intramolecular [2+2] Cycloaddition of N‐alkyl‐N‐(2‐(1‐arylvinyl)aryl)cinnamamides

Weber Paixão, Márcio ; de Souza, Wanderson ; Matsuo, Bianca ; Matos, Priscilla ; Correia Correia, José Tiago M. ; Santos, Marilia S. ; König, Burkhard



Abstract

N ‐Alkyl‐ N ‐(2‐(1‐arylvinyl)aryl)cinnamamides are converted into natural product inspired scaffolds via iridium photocatalyzed intramolecular [2+2] photocycloaddition. The protocol has a broad substrate scope, whilst operating under mild reaction conditions. Tethering four components forming a trisubstituted cyclobutane core builds rapidly high molecular complexity. Our approach allows the ...

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