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All-organic Z-scheme photoreduction of CO2 with water as the donor of electrons and protons

Mazzanti, Stefano ; Cao, Shaowen ; Brummelhuis, Katharina ten ; Völkel, Antje ; Khamrai, Jagadish ; Sharapa, Dmitry I. ; Youk, Sol ; Heil, Tobias ; Tarakina, Nadezda V. ; Strauss, Volker ; Ghosh, Indrajit ; König, Burkhard ; Oschatz, Martin ; Antonietti, Markus ; Savateev, Aleksandr


Carbon nitrides and flavins are two classes of easy accessible transition metal-free, photoactive materials. Their photocatalytic efficiency to enable a variety of chemical reactions is well documented. Here, we report on their combination in one photocatalytic system by designing biomimetic non-spherical core-shell architectures comprising micro-sized crystals of flavins decorated by potassium ...


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