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Elucidation of the Intersystem Crossing Mechanism in a Helical BODIPY for Low-Dose Photodynamic Therapy

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Wang, Zhijia ; Huang, Ling ; El‐Zohry, Ahmed M. ; Dick, Bernhard ; ; ; ; ; ;
Date of publication of this fulltext: 25 Jan 2021 07:50

This publication is part of the DEAL contract with Wiley.


Intersystem crossing (ISC) of triplet photosensitizers is a vital process for fundamental photochemistry and photodynamic therapy (PDT). Herein, we report the co-existence of efficient ISC and long triplet excited lifetime in a heavy atomfree bodipy helicene molecule. Via theoretical computation and time-resolved EPR spectroscopy, we confirmed that the ISC of the bodipy results from its twisted ...


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