Direkt zum Inhalt

Krause, Razvan ; Chávez-Cervantes, Mariana ; Aeschlimann, Sven ; Forti, Stiven ; Fabbri, Filippo ; Rossi, Antonio ; Coletti, Camilla ; Cacho, Cephise ; Zhang, Yu ; Majchrzak, Paulina Ewa ; Chapman, Richard T. ; Springate, Emma ; Gierz, Isabella

Ultrafast Charge Separation in Bilayer WS2/Graphene Heterostructure Revealed by Time- and Angle-Resolved Photoemission Spectroscopy

Krause, Razvan, Chávez-Cervantes, Mariana, Aeschlimann, Sven, Forti, Stiven, Fabbri, Filippo , Rossi, Antonio, Coletti, Camilla , Cacho, Cephise, Zhang, Yu , Majchrzak, Paulina Ewa , Chapman, Richard T., Springate, Emma und Gierz, Isabella (2021) Ultrafast Charge Separation in Bilayer WS2/Graphene Heterostructure Revealed by Time- and Angle-Resolved Photoemission Spectroscopy. Frontiers in Physics 2021 (9), S. 668149. (Eingereicht)

Veröffentlichungsdatum dieses Volltextes: 01 Jun 2021 15:15
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.44995


Zusammenfassung

Efficient light harvesting devices need to combine strong absorption in the visible spectral range with efficient ultrafast charge separation. These features commonly occur in novel ultimately thin van der Waals heterostructures with type II band alignment. Recently, ultrafast charge separation was also observed in monolayer WS2/graphene heterostructures with type I band alignment. Here we use ...

Efficient light harvesting devices need to combine strong absorption in the visible spectral range with efficient ultrafast charge separation. These features commonly occur in novel ultimately thin van der Waals heterostructures with type II band alignment. Recently, ultrafast charge separation was also observed in monolayer WS2/graphene heterostructures with type I band alignment. Here we use time- and angle-resolved photoemission spectroscopy to show that ultrafast charge separation also occurs at the interface between bilayer WS2 and graphene indicating that the indirect band gap of bilayer WS2 does not affect the charge transfer to the graphene layer. The microscopic insights gained in the present study will turn out to be useful for the design of novel optoelectronic devices.



Beteiligte Einrichtungen


Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftFrontiers in Physics
Verlag:Frontiers
Ort der Veröffentlichung:LAUSANNE
Band:2021
Nummer des Zeitschriftenheftes oder des Kapitels:9
Seitenbereich:S. 668149
Datum29 April 2021
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Prof. Dr. Isabella Gierz
Identifikationsnummer
WertTyp
10.3389/fphy.2021.668149DOI
Stichwörter / KeywordsEXCITON BINDING-ENERGY; BANDGAP RENORMALIZATION; GRAPHENE; LAYERS; TMD; graphene; van der Waals heterostructures; tr-ARPES; ultrafast charge transfer; photovoltaics
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusEingereicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenJa
URN der UB Regensburgurn:nbn:de:bvb:355-epub-449955
Dokumenten-ID44995

Bibliographische Daten exportieren

Nur für Besitzer und Autoren: Kontrollseite des Eintrags

nach oben