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Ultrafast Charge Separation in Bilayer WS2/Graphene Heterostructure Revealed by Time- and Angle-Resolved Photoemission Spectroscopy
Krause, Razvan, Chávez-Cervantes, Mariana, Aeschlimann, Sven, Forti, Stiven, Fabbri, Filippo
, Rossi, Antonio, Coletti, Camilla
, Cacho, Cephise, Zhang, Yu
, Majchrzak, Paulina Ewa
, Chapman, Richard T., Springate, Emma
und Gierz, Isabella
(2021)
Ultrafast Charge Separation in Bilayer WS2/Graphene Heterostructure Revealed by Time- and Angle-Resolved Photoemission Spectroscopy.
Frontiers in Physics 2021 (9), S. 668149.
(Eingereicht)
Veröffentlichungsdatum dieses Volltextes: 01 Jun 2021 15:15
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.44995
Zusammenfassung
Efficient light harvesting devices need to combine strong absorption in the visible spectral range with efficient ultrafast charge separation. These features commonly occur in novel ultimately thin van der Waals heterostructures with type II band alignment. Recently, ultrafast charge separation was also observed in monolayer WS2/graphene heterostructures with type I band alignment. Here we use ...
Efficient light harvesting devices need to combine strong absorption in the visible spectral range with efficient ultrafast charge separation. These features commonly occur in novel ultimately thin van der Waals heterostructures with type II band alignment. Recently, ultrafast charge separation was also observed in monolayer WS2/graphene heterostructures with type I band alignment. Here we use time- and angle-resolved photoemission spectroscopy to show that ultrafast charge separation also occurs at the interface between bilayer WS2 and graphene indicating that the indirect band gap of bilayer WS2 does not affect the charge transfer to the graphene layer. The microscopic insights gained in the present study will turn out to be useful for the design of novel optoelectronic devices.
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| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Frontiers in Physics | ||||
| Verlag: | Frontiers | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | LAUSANNE | ||||
| Band: | 2021 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 9 | ||||
| Seitenbereich: | S. 668149 | ||||
| Datum | 29 April 2021 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Prof. Dr. Isabella Gierz | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | EXCITON BINDING-ENERGY; BANDGAP RENORMALIZATION; GRAPHENE; LAYERS; TMD; graphene; van der Waals heterostructures; tr-ARPES; ultrafast charge transfer; photovoltaics | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Eingereicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-449955 | ||||
| Dokumenten-ID | 44995 |
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