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Defluorodearomatization: A Photocatalytic Birch-Like Reduction That Enables C–C Bond Formation and Provides Access to Unnatural Cannabinoids

Day, Jon I. ; Grotjahn, Sascha ; Senaweera, Sameera ; König, Burkhard ; Weaver, Jimmie D.



Abstract

Within the framework of discovery chemistry, polyfluorination remains a synthetic challenge despite its ability to provide useful characteristics, such as a reduction in the number of hydrogen bond donors and metabolic stability. Coupling a reversal of this methodology with photocatalysis has been demonstrated to allow the rapid synthesis of previously difficult or impossible targets by starting ...

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