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Electrochemical gate-controlled electron transport of redox-active single perylene bisimide molecular junctions

Li, C. ; Mishchenko, A. ; Li, Z. ; Pobelov, I. ; Wandlowski, Th. ; Li, X. Q. ; Würthner, F. ; Bagrets, A. ; Evers, Ferdinand


We report a scanning tunneling microscopy (STM) experiment in an electrochemical environment which studies a prototype molecular switch. The target molecules were perylene tetracarboxylic acid bisimides modified with pyridine (P-PBI) and methylthiol (T-PBI) linker groups and with bulky tert-butyl-phenoxy substituents in the bay area. At a fixed bias voltage, we can control the transport current ...


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