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Atomically resolved single-molecule triplet quenching

Peng, Jinbo ; Sokolov, Sophia ; Hernangómez-Pérez, Daniel ; Evers, Ferdinand ; Gross, Leo ; Lupton, John M. ; Repp, Jascha


The nonequilibrium triplet state of molecules plays an important role in photocatalysis, organic photovoltaics, and photodynamic therapy. We report the direct measurement of the triplet lifetime of an individual pentacene molecule on an insulating surface with atomic resolution by introducing an electronic pumpprobe method in atomic force microscopy. Strong quenching of the triplet lifetime is ...


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