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Excited-State Switching between Ligand-Centered and Charge Transfer Modulated by Metal–Carbon Bonds in Cyclopentadienyl Iridium Complexes

Deaton, Joseph C. ; Taliaferro, Chelsea M. ; Pitman, Catherine L. ; Czerwieniec, Rafał ; Jakubikova, Elena ; Miller, Alexander J. M. ; Castellano, Felix N.



Zusammenfassung

Three series of pentamethylcyclopentadienyl (Cp*) Ir(III) complexes with different bidentate ligands were synthesized and structurally characterized, [Cp*Ir(tpy)L](n+) (tpy = 2-tolylpyridinato; n = 0 or 1), [Cp*Ir(piq)L](n+) (piq = 1-phenylisoquinolinato; n = 0 or 1), and [Cp*Ir(bpy)L](m+) (bpy = 2,2'-bipyridine; m = 1 or 2), featuring a range of monodentate carbon -donor ligands within each ...

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