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Fluorine as a Traceless Directing Group for the Regiodivergent Synthesis of Indoles and Tryptophans

Andries-Ulmer, Anna ; Brunner, Christoph ; Rehbein, Julia ; Gulder, Tanja


Despite ample evidence for the unique reactivity offered by hypervalent F-iodanes, mechanistic investigations fall far behind. In order to shed light on the unusual behavior of such F-reagents, we conducted computational and experimental studies on the chemodivergent transformation of styrenes. We identified the spirocyclic F-cyclopropane as the common intermediate for both the C,H-fluorination ...


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