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Visible‐Light‐Accelerated Copper(II)‐Catalyzed Regio‐ and Chemoselective Oxo‐Azidation of Vinyl Arenes

Hossain, Asik ; Vidyasagar, Adiyala ; Eichinger, Christian ; Lankes, Christian ; Phan, Jenny ; Rehbein, Julia ; Reiser, Oliver



Abstract

The visible-light-accelerated oxo-azidation of vinyl arenes with trimethylsilylazide and molecular oxygen as stoichiometric oxidant was achieved. In contrast to photocatalysts based on iridium, ruthenium, or organic dyes, [Cu(dap)(2)]Cl or [Cu(dap)Cl-2] were found to be unique for this transformation, which is attributed to their ability to interact with the substrates through ligand exchange and ...

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