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Internal acidity scale and reactivity evaluation of chiral phosphoric acids with different 3,3′-substituents in Brønsted acid catalysis

Rothermel, Kerstin ; Melikian, Maxime ; Hioe, Johnny ; Greindl, Julian ; Gramüller, Johannes ; Žabka, Matej ; Sorgenfrei, Nils ; Hausler, Thomas ; Morana, Fabio ; Gschwind, Ruth M.


The concept of hydrogen bonding for enhancing substrate binding and controlling selectivity and reactivity is central in catalysis. However, the properties of these key hydrogen bonds and their catalyst-dependent variations are extremely difficult to determine directly by experiments. Here, for the first time the hydrogen bond properties of a whole series of BINOL-derived chiral phosphoric acid ...


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