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Sky-blue thermally activated delayed fluorescence (TADF) based on Ag(i) complexes: strong solvation-induced emission enhancement

Artem'ev, Alexander V. ; Shafikov, Marsel Z. ; Schinabeck, Alexander ; Antonova, Olga V. ; Berezin, Alexey S. ; Bagryanskaya, Irina Yu. ; Plusnin, Pavel E. ; Yersin, Hartmut



Abstract

A new Ag(I) complex based on tris(2-pyridyl)phosphine (Py3P), [Ag-2(Py3P)(3)(SCN)(2)], has been synthesized and chemically characterized. Theoretical calculations and photophysical investigations reveal thermally activated delayed fluorescence (TADF) coupled with outstanding solvato- and vapor-luminescent behavior. The parent complex [Ag-2(Py3P)(3)(SCN)(2)] shows sky-blue TADF (lambda(max) = 469 ...

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