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CO2 activation by manganese pincer complexes through different modes of metal–ligand cooperation

Kumar, Amit ; Daw, Prosenjit ; Espinosa-Jalapa, Noel Angel ; Leitus, Gregory ; Shimon, Linda J. W. ; Ben-David, Yehoshoa ; Milstein, David


We report here the activation of CO2 using two Mn-PNN pincer complexes that can exhibit different modes of metal-ligand cooperation amido/amino mode that involves [1,2]-activation of CO2 and dearomatization/aromatization mode that involves [1,3]-activation of CO2. We also compare their catalytic activity for CO2 hydrogenation.

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