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Visible-Light-Mediated Regioselective Chlorosulfonylation of Alkenes and Alkynes: Introducing the Cu(II) Complex [Cu(dap)Cl2] to Photochemical ATRA Reactions

Hossain, Asik ; Engl, Sebastian ; Lutsker, Eugen ; Reiser, Oliver



Abstract

A visible-light-mediated photocatalyzed protocol utilizing copper-phenanthroline-based catalysts has been developed that can convert a large number of olefins into their chlorosulfonylated products. Besides the Cu(I) complex [Cu(dap)(2)]Cl, now well-established in photo-ATRA processes, the corresponding Cu(II) complex [Cu(dap)Cl-2] proved to be often even more efficient in the title reaction, ...

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