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Redox Noninnocent Nature of Acridine-Based Pincer Complexes of 3d Metals and C–C Bond Formation

Daw, Prosenjit ; Kumar, Amit ; Oren, Dror ; Espinosa-Jalapa, Noel Angel ; Srimani, Dipankar ; Diskin-Posner, Yael ; Leitus, Gregory ; Shimon, Linda J. W. ; Carmieli, Raanan ; Ben-David, Yehoshoa ; Milstein, David



Abstract

Acridine-based PNP pincer complexes have been previously utilized for several environmentally benign catalytic processes. In light of the recent growth in interest in base-metal catalysis, we report here the synthesis of acridine-PNP pincer complexes of Ni, Co, Fe, and Mn. We also report here the noninnocent redox nature of these complexes that results in the dimerization of pincer complexes by forming a C-C bond at the C9 position of the acridine ring.


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