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Spin–Orbit Charge‐Transfer Intersystem Crossing (ISC) in Compact Electron Donor–Acceptor Dyads: ISC Mechanism and Application as Novel and Potent Photodynamic Therapy Reagents

Wang, Zhijia ; Ivanov, Mikhail ; Gao, Yuting ; Bussotti, Laura ; Foggi, Paolo ; Zhang, Huimin ; Russo, Nino ; Dick, Bernhard ; Zhao, Jianzhang ; Di Donato, Mariangela ; Mazzone, Gloria ; Luo, Liang ; Fedin, Matvey


Spin-orbit charge-transfer intersystem crossing (SOCT-ISC) is useful for the preparation of heavy atom-free triplet photosensitisers (PSs). Herein, a series of perylene-Bodipy compact electron donor/acceptor dyads showing efficient SOCT-ISC is prepared. The photophysical properties of the dyads were studied with steady-state and time-resolved spectroscopies. Efficient triplet state formation ...


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