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Exploiting Cooperative Catalysis for the On-surface Synthesis of Linear Heteroaromatic Polymers via Selective C-H Activation

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Liu, Xunshan ; Matej, Adam ; Kratky, Tim ; Mendieta-Moreno, Jesús I. ; Günther, Sebastian ; Mutombo, Pingo ; Decurtins, Silvio ; Aschauer, Ulrich ; Repp, Jascha ; Jelinek, Pavel ; Liu, Shi-Xia ; Patera, Laerte L.
Date of publication of this fulltext: 02 Dec 2021 05:42


Regiospecific C-H activation is a promising approach to achieve extended polymers with tailored structures. While a recent on-surface synthetic approach has enabled regioselective homocoupling of heteroaromatic molecules, only small oligomers have been achieved. Herein, selective C-H activation for dehydrogenative C-C couplings of hexaazatriphenylene by Scholl reaction is reported for the first ...


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