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Meineke, Christian ; Prager, Michael ; Hayes, Johannes ; Wen, Qiannan ; Kastner, Lukas Zheyi ; Schuh, Dieter ; Fritsch, Kilian ; Pronin, Oleg ; Stein, Markus ; Schäfer, Felix ; Chatterjee, Sangam ; Kira, Mackillo ; Huber, Rupert ; Bougeard, Dominique

Scalable high-repetition-rate sub-half-cycle terahertz pulses from spatially indirect interband transitions

Meineke, Christian , Prager, Michael , Hayes, Johannes , Wen, Qiannan, Kastner, Lukas Zheyi , Schuh, Dieter, Fritsch, Kilian, Pronin, Oleg , Stein, Markus, Schäfer, Felix , Chatterjee, Sangam, Kira, Mackillo, Huber, Rupert and Bougeard, Dominique (2022) Scalable high-repetition-rate sub-half-cycle terahertz pulses from spatially indirect interband transitions. Light: Science & Applications 11, art.no.151.

Date of publication of this fulltext: 31 May 2022 05:35
Article
DOI to cite this document: 10.5283/epub.52338


Abstract

Intense phase-locked terahertz (THz) pulses are the bedrock of THz lightwave electronics, where the carrier field creates a transient bias to control electrons on sub-cycle time scales. Key applications such as THz scanning tunnelling microscopy or electronic devices operating at optical clock rates call for ultimately short, almost unipolar waveforms, at megahertz (MHz) repetition rates. Here, ...

Intense phase-locked terahertz (THz) pulses are the bedrock of THz lightwave electronics, where the carrier field creates a transient bias to control electrons on sub-cycle time scales. Key applications such as THz scanning tunnelling microscopy or electronic devices operating at optical clock rates call for ultimately short, almost unipolar waveforms, at megahertz (MHz) repetition rates. Here, we present a flexible and scalable scheme for the generation of strong phase-locked THz pulses based on shift currents in type-II-aligned epitaxial semiconductor heterostructures. The measured THz waveforms exhibit only 0.45 optical cycles at their centre frequency within the full width at half maximum of the intensity envelope, peak fields above 1.1 kV cm(-1) and spectral components up to the mid-infrared, at a repetition rate of 4 MHz. The only positive half-cycle of this waveform exceeds all negative half-cycles by almost four times, which is unexpected from shift currents alone. Our detailed analysis reveals that local charging dynamics induces the pronounced positive THz-emission peak as electrons and holes approach charge neutrality after separation by the optical pump pulse, also enabling ultrabroadband operation. Our unipolar emitters mark a milestone for flexibly scalable, next-generation high-repetition-rate sources of intense and strongly asymmetric electric field transients.



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Item typeArticle
Journal or Publication TitleLight: Science & Applications
Publisher:Springer
Open Access Type:DEAL (Springer Gold)
Place of Publication:LONDON
Volume:11
Page Range:art.no.151
Date23 May 2022
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Rupert Huber
Physics > Institute of Experimental and Applied Physics > Chair Professor Huber > Group Dominique Bougeard
Identification Number
ValueType
10.1038/s41377-022-00824-6DOI
KeywordsSINGLE-MOLECULE; EMITTERS; LIGHT; FIELD
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgPartially
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-523385
Item ID52338

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