Direkt zum Inhalt

Meineke, Christian ; Prager, Michael ; Hayes, Johannes ; Wen, Qiannan ; Kastner, Lukas Zheyi ; Schuh, Dieter ; Fritsch, Kilian ; Pronin, Oleg ; Stein, Markus ; Schäfer, Felix ; Chatterjee, Sangam ; Kira, Mackillo ; Huber, Rupert ; Bougeard, Dominique

Scalable high-repetition-rate sub-half-cycle terahertz pulses from spatially indirect interband transitions

Meineke, Christian , Prager, Michael , Hayes, Johannes , Wen, Qiannan, Kastner, Lukas Zheyi , Schuh, Dieter, Fritsch, Kilian, Pronin, Oleg , Stein, Markus, Schäfer, Felix , Chatterjee, Sangam, Kira, Mackillo, Huber, Rupert und Bougeard, Dominique (2022) Scalable high-repetition-rate sub-half-cycle terahertz pulses from spatially indirect interband transitions. Light: Science & Applications 11, art.no.151.

Veröffentlichungsdatum dieses Volltextes: 31 Mai 2022 05:35
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.52338


Zusammenfassung

Intense phase-locked terahertz (THz) pulses are the bedrock of THz lightwave electronics, where the carrier field creates a transient bias to control electrons on sub-cycle time scales. Key applications such as THz scanning tunnelling microscopy or electronic devices operating at optical clock rates call for ultimately short, almost unipolar waveforms, at megahertz (MHz) repetition rates. Here, ...

Intense phase-locked terahertz (THz) pulses are the bedrock of THz lightwave electronics, where the carrier field creates a transient bias to control electrons on sub-cycle time scales. Key applications such as THz scanning tunnelling microscopy or electronic devices operating at optical clock rates call for ultimately short, almost unipolar waveforms, at megahertz (MHz) repetition rates. Here, we present a flexible and scalable scheme for the generation of strong phase-locked THz pulses based on shift currents in type-II-aligned epitaxial semiconductor heterostructures. The measured THz waveforms exhibit only 0.45 optical cycles at their centre frequency within the full width at half maximum of the intensity envelope, peak fields above 1.1 kV cm(-1) and spectral components up to the mid-infrared, at a repetition rate of 4 MHz. The only positive half-cycle of this waveform exceeds all negative half-cycles by almost four times, which is unexpected from shift currents alone. Our detailed analysis reveals that local charging dynamics induces the pronounced positive THz-emission peak as electrons and holes approach charge neutrality after separation by the optical pump pulse, also enabling ultrabroadband operation. Our unipolar emitters mark a milestone for flexibly scalable, next-generation high-repetition-rate sources of intense and strongly asymmetric electric field transients.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftLight: Science & Applications
Verlag:Springer
Ort der Veröffentlichung:LONDON
Band:11
Seitenbereich:art.no.151
Datum23 Mai 2022
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Dominique Bougeard
Identifikationsnummer
WertTyp
10.1038/s41377-022-00824-6DOI
Stichwörter / KeywordsSINGLE-MOLECULE; EMITTERS; LIGHT; FIELD
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-523385
Dokumenten-ID52338

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