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Selectivity in single-molecule reactions by tip-induced redox chemistry

Albrecht, Florian ; Fatayer, Shadi ; Pozo, Iago ; Tavernelli, Ivano ; Repp, Jascha ; Peña, Diego ; Gross, Leo



Abstract

Controlling selectivity of reactions is an ongoing quest in chemistry. In this work, we demonstrate reversible and selective bond formation and dissociation promoted by tip-induced reduction-oxidation reactions on a surface. Molecular rearrangements leading to different constitutional isomers are selected by the polarity and magnitude of applied voltage pulses from the tip of a combined scanning ...

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