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Bidentate Substrate Binding in Brønsted Acid Catalysis: Structural Space, Hydrogen Bonding and Dimerization

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Gramüller, Johannes ; Dullinger, Philipp ; Horinek, Dominik ; Gschwind, Ruth M.
Date of publication of this fulltext: 19 Dec 2022 09:35


BINOL derived chiral phosphoric acids (CPAs) are a prominent class of catalysts in the field of asymmetric organocatalysis, capable of transforming a wide selection of substrates with high stereoselectivities. Exploiting the Brønsted acidic and basic dual functionality of CPAs, substrates with both a hydrogen bond acceptor and donor functionality are frequently used as the resulting bidentate ...


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