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Superlinear Photogalvanic Effects in (Bi0.3Sb0.7)2(Te0.1Se0.9)3: Probing Three-Dimensional Topological Insulator Surface States at Room Temperature
Danilov, Sergey N.
, Golub, Leonid E.
, Mayer, T., Beer, A.
, Binder, Stefan
, Mönch, E., Minár, J., Kronseder, Matthias
, Back, Christian H.
, Bougeard, Dominique
und Ganichev, Sergey D.
(2021)
Superlinear Photogalvanic Effects in (Bi0.3Sb0.7)2(Te0.1Se0.9)3: Probing Three-Dimensional Topological Insulator Surface States at Room Temperature.
Physical Review Applied 16 (6), 064030.
Veröffentlichungsdatum dieses Volltextes: 15 Feb 2023 16:44
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.53798
Zusammenfassung
We report on the observation of a complex nonlinear intensity dependence of the circular and linear photogalvanic currents induced by infrared radiation in compensated (Bi0.3Sb0.7)(2) (Te0.1Se0.9)(3) three-dimensional topological insulators. The photocurrents are induced by direct optical transitions between topological surface and bulk states. We show that an increase in the radiation intensity ...
We report on the observation of a complex nonlinear intensity dependence of the circular and linear photogalvanic currents induced by infrared radiation in compensated (Bi0.3Sb0.7)(2) (Te0.1Se0.9)(3) three-dimensional topological insulators. The photocurrents are induced by direct optical transitions between topological surface and bulk states. We show that an increase in the radiation intensity results first in a highly superlinear rise in the amplitude of both types of photocurrents, whereas at higher intensities the photocurrent saturates. Our analysis of the observed nonlinearities shows that the superlinear behavior of the photocurrents is caused by heating of the electron gas, while the saturation is induced by slow relaxation of the photoexcited carriers, resulting in absorbance bleaching. The observed nonlinearities give access to the Fermi-level position with respect to the Dirac point and the energy relaxation times of Dirac fermions, providing an experimental room-temperature probe of topological surface states.
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| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Physical Review Applied | ||||
| Verlag: | AMER PHYSICAL SOC | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | COLLEGE PK | ||||
| Band: | 16 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 6 | ||||
| Seitenbereich: | 064030 | ||||
| Datum | 13 Dezember 2021 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Entpflichtete oder im Ruhestand befindliche Professoren > Lehrstuhl Professor Back > Arbeitsgruppe Christian Back Physik > Institut für Experimentelle und Angewandte Physik > Professor Ganichev > Arbeitsgruppe Sergey Ganichev Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Dominique Bougeard Physik > Institut für Experimentelle und Angewandte Physik > Prof. Jörg Wunderlich | ||||
| Identifikationsnummer |
| ||||
| Stichwörter / Keywords | SPIN PHOTOCURRENTS; DEEP IMPURITIES; SPECTROSCOPY; IONIZATION; BI2SE3; BI2TE3 | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-537988 | ||||
| Dokumenten-ID | 53798 |
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