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Link between interlayer hybridization and ultrafast charge transfer in WS2-graphene heterostructures

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Hofmann, Niklas ; Weigl, Leonard ; Gradl, Johannes ; Mishra, Neeraj ; Orlandini, Giorgio ; Forti, Stiven ; Coletti, Camilla ; Latini, Simone ; Xian, Lede ; Rubio, Angel ; Paredes, Dilan Perez ; Causin, Raul Perea ; Brem, Samuel ; Malic, Ermin ; Gierz, Isabella
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Date of publication of this fulltext: 23 Oct 2023 11:38


Ultrafast charge separation after photoexcitation is a common phenomenon in various van-der-Waals (vdW) heterostructures with great relevance for future applications in light harvesting and detection. Theoretical understanding of this phenomenon converges towards a coherent mechanism through charge transfer states accompanied by energy dissipation into strongly coupled phonons. The detailed ...


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