Nonlinear spectroscopic studies using sum- and difference-frequency generation

URN to cite this document:: urn:nbn:de:bvb:355-epub-55171
DOI to cite this document:: 10.5283/epub.5517

Dick, Bernhard ; Hochstrasser, R. M.

Preview

PDF
(920kB)

Date of publication of this fulltext: 05 Aug 2009 13:50

Alternative links to fulltext:DOI

Details

Preview

Export bibliographical data

Abstract

A detailed study is presented of resonant sum- and difference-frequency generation for the mixed-crystal system azulene in naphthalene. The S0 -> S1, S0 -> S2 and S1 -> S2 transitions of azulene provide the 3 needed dipoles for the existence of c(2), and a relatively small static elec. field was used to break the interference between the waves generated in the 2 crystal sublattices. Second-order ...