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Di-tert-butyldiphosphatetrahedrane as a building block for phosphaalkenes and phosphirenes

Hierlmeier, Gabriele ; Uttendorfer, Maria K. ; Wolf, Robert



Abstract

The remarkable 'mixed' diphosphatetrahedrane (tBuCP)(2) (1) - which is both the elusive dimeric form of the phosphaalkyne tBuCP and an isolobal analogue of the important industrial feedstock P-4 - was recently isolated for the first time; however, its chemistry remains unexplored. Herein we report that treatment of 1 with various N-heterocyclic carbenes readily yields unusual, unsaturated ...

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