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Nonlinear spectroscopy of excitonic states in transition metal dichalcogenides

Zhumagulov, Yaroslav V. ; Neverov, Vyacheslav D. ; Lukyanov, Alexander E. ; Gulevich, Dmitry R. ; Krasavin, Andrey V. ; Vagov, Alexei ; Perebeinos, Vasili


Second-harmonic generation (SHG) is a well-known nonlinear spectroscopy method to probe electronic structure, specifically, in transition metal dichalcogenide (TMDC) monolayers. This work investigates the nonlinear dynamics of a strongly excited TMDC monolayer by solving the time evolution equations for the density matrix. It is shown that the presence of excitons qualitatively changes the ...


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