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Aeschlimann, Martin ; Bange, Jan Philipp ; Bauer, Michael ; Bovensiepen, Uwe ; Elmers, Hans-Joachim ; Fauster, Thomas ; Gierster, Lukas ; Höfer, Ulrich ; Huber, Rupert ; Li, Andi ; Li, Xitong ; Mathias, Stefan ; Morgenstern, Karina ; Petek, Hrvoje ; Reutzel, Marcel ; Rossnagel, Kai ; Schönhense, Gerd ; Scholz, Markus ; Stadtmüller, Benjamin ; Stähler, Julia ; Tan, Shijing ; Wang, Bing ; Wang, Zehua ; Weinelt, Martin

Time-resolved photoelectron spectroscopy at surfaces

Aeschlimann, Martin , Bange, Jan Philipp, Bauer, Michael, Bovensiepen, Uwe, Elmers, Hans-Joachim , Fauster, Thomas , Gierster, Lukas, Höfer, Ulrich, Huber, Rupert , Li, Andi, Li, Xitong, Mathias, Stefan, Morgenstern, Karina, Petek, Hrvoje, Reutzel, Marcel, Rossnagel, Kai , Schönhense, Gerd, Scholz, Markus, Stadtmüller, Benjamin, Stähler, Julia, Tan, Shijing, Wang, Bing, Wang, Zehua und Weinelt, Martin (2024) Time-resolved photoelectron spectroscopy at surfaces. Surface Science 753 (12263).

Veröffentlichungsdatum dieses Volltextes: 12 Dez 2024 07:41
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.59784


Zusammenfassung

Light is a preeminent spectroscopic tool for investigating the electronic structure of surfaces. Time-resolved photoelectron spectroscopy has mainly been developed in the last 30 years. It is therefore not surprising that the topic was hardly mentioned in the issue on “The first thirty years” of surface science. In the second thirty years, however, we have seen tremendous progress in the ...

Light is a preeminent spectroscopic tool for investigating the electronic structure of surfaces. Time-resolved photoelectron spectroscopy has mainly been developed in the last 30 years. It is therefore not surprising that the topic was hardly mentioned in the issue on “The first thirty years” of surface science. In the second thirty years, however, we have seen tremendous progress in the development of time-resolved photoelectron spectroscopy on surfaces. Femtosecond light pulses and advanced photoelectron detection schemes are increasingly being used to study the electronic structure and dynamics of occupied and unoccupied electronic states and dynamic processes such as the energy and momentum relaxation of electrons, charge transfer at interfaces and collective processes such as plasmonic excitation and optical field screening. Using spin- and time-resolved photoelectron spectroscopy, we were able to study ultrafast spin dynamics, electron–magnon scattering and spin structures in magnetic and topological materials. Light also provides photon energy as well as electric and magnetic fields that can influence molecular surface processes to steer surface photochemistry and hot-electron-driven catalysis. In addition, we can consider light as a chemical reagent that can alter the properties of matter by creating non-equilibrium states and ultrafast phase transitions in correlated materials through the coupling of electrons, phonons and spins. Electric fields have also been used to temporarily change the electronic structure. This opened up new methods and areas such as high harmonic generation, light wave electronics and attosecond physics. This overview certainly cannot cover all these interesting topics. But also as a testimony to the cohesion and constructive exchange in our ultrafast community, a number of colleagues have come together to share their expertise and views on the very vital field of dynamics at surfaces. Following the introduction, the interested reader will find a list of contributions and a brief summary in Section 1.3.



Beteiligte Einrichtungen


Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftSurface Science
Verlag:Elsevier
Band:753
Nummer des Zeitschriftenheftes oder des Kapitels:12263
Datum1 November 2024
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Identifikationsnummer
WertTyp
10.1016/j.susc.2024.122631DOI
Stichwörter / KeywordsTime-resolved photoemission, Image-potential states, Time-resolved photoemission electron microscopy, Hot electron dynamics, Plasmons, Semiconductor heterostructures, Photostationary states, Time-and spin-resolved photoemission, Ultrafast spin dynamics, Magnons, Femtomagnetism, Time-resolved momentum microscopy, Exciton dynamics, Dark exciton, Interlayer exciton, Intervalley scattering, Momentum microscope, Scherzer theorem, Free-electron laser
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
Dokumenten-ID59784

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