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Pump-induced population changes in broadband coherent anti-Stokes Raman scattering

Gierulski, A., Noda, M., Yamamoto, T., Marowsky, G. and Slenczka, A. (1987) Pump-induced population changes in broadband coherent anti-Stokes Raman scattering. Optics Letters 12 (8), pp. 608-10.

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Bu using a powerful, excimer-laser-pumped broadband CARS system, considerable changes were obsd. in the populations of room-temp. N2 under atm. pressure. Pump-induced populations in the 1st, 2nd, and 3rd vibronic bands of N2 at room temp. resulted in an apparent vibrational temp. of 2550 K. The implications for broadband N2 CARS thermometry are discussed.

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Item type:Article
Additional Information (public):CAN 107:123571; 73-3; Optical, Electron, and Mass Spectroscopy and Other Related Properties; 7727-37-9 (Nitrogen) Role: PRP (Properties) (pump induced population changes in broadband CARS of, temp. detn. in relation to)
Institutions:Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry III - Physical Chemistry (Molecular Spectroscopy and Photochemistry) > Prof. Dr. Alkwin Slenczka
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Keywords:Temperature (detn. of, CARS of nitrogen in); Raman spectrometry (CARS, in temp. detn.); CARS nitrogen thermometry; Raman nitrogen thermometry
Dewey Decimal Classification:500 Science > 530 Physics
500 Science > 540 Chemistry & allied sciences
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:No
Item ID:6061
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