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Immobilised Zinc (II) Cyclen complexes as catalytic reagents for phosphodiester hydrolysis

Walenzyk, T. and Koenig, B. (2005) Immobilised Zinc (II) Cyclen complexes as catalytic reagents for phosphodiester hydrolysis. Inorg. Chim. Acta 358, 2269 - 2274.

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Many hydrolases found in nature have Zn(II) ions at their active site. Artificial hydrolases as alternatives for non-enzymatic hydrolysis were prepared by attaching Zn(II) cyclen complexes with an alcohol pendant to a polymeric support. These modified polymers showed a 104-fold enhanced intrinsic reactivity for the hydrolysis of activated phosphodiesters over the non-catalysed reaction
in solution.

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Item type:Article
Institutions:Chemistry and Pharmacy > Institut für Organische Chemie > Lehrstuhl Prof. Dr. Burkhard König
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Keywords:Phosphoester hydrolysis; Immobilised metal complexes; Zinc (II) cyclen
Dewey Decimal Classification:500 Science > 540 Chemistry & allied sciences
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Item ID:6248
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