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Crossover from Nonthermal to Thermal Photoluminescence from Metals Excited by Ultrashort Light Pulses
Sivan, Yonatan, Un, Ieng Wai, Kalyan, Imon, Lin, Kai-Qiang
, Lupton, John M.
und Bange, Sebastian
(2023)
Crossover from Nonthermal to Thermal Photoluminescence from Metals Excited by Ultrashort Light Pulses.
ACS Nano 17 (12), S. 11439-11453.
Veröffentlichungsdatum dieses Volltextes: 11 Mrz 2025 13:33
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.75215
Zusammenfassung
Photoluminescence from metal nanostructures following intense ultrashort illumination is a fundamental aspect of light–matter interactions. Surprisingly, many of its basic characteristics are under ongoing debate. Here, we resolve many of these debates by providing a comprehensive theoretical framework that describes this phenomenon and support it by an experimental confirmation. Specifically, we ...
Photoluminescence from metal nanostructures following intense ultrashort illumination is a fundamental aspect of light–matter interactions. Surprisingly, many of its basic characteristics are under ongoing debate. Here, we resolve many of these debates by providing a comprehensive theoretical framework that describes this phenomenon and support it by an experimental confirmation. Specifically, we identify aspects of the emission that are characteristic to either nonthermal or thermal emission, in particular, differences in the spectral and electric field dependence of these two contributions to the emission. Overall, nonthermal emission is characteristic of the early stages of light emission, while the later stages show thermal characteristics. The former dominate only for moderately high illumination intensities for which the electron temperature reached after thermalization remains close to room temperature.
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| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | ACS Nano | ||||
| Verlag: | American Chemical Society (ACS) | ||||
|---|---|---|---|---|---|
| Band: | 17 | ||||
| Nummer des Zeitschriftenheftes oder des Kapitels: | 12 | ||||
| Seitenbereich: | S. 11439-11453 | ||||
| Datum | 8 Juni 2023 | ||||
| Institutionen | Physik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe John Lupton | ||||
| Identifikationsnummer |
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| Stichwörter / Keywords | plasmonics, electron nonequilibrium, photoluminescence, thermo-optic effects, metal nanoparticles | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Zum Teil | ||||
| Dokumenten-ID | 75215 |
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