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Sivan, Yonatan ; Un, Ieng Wai ; Kalyan, Imon ; Lin, Kai-Qiang ; Lupton, John M. ; Bange, Sebastian

Crossover from Nonthermal to Thermal Photoluminescence from Metals Excited by Ultrashort Light Pulses

Sivan, Yonatan, Un, Ieng Wai, Kalyan, Imon, Lin, Kai-Qiang , Lupton, John M. und Bange, Sebastian (2023) Crossover from Nonthermal to Thermal Photoluminescence from Metals Excited by Ultrashort Light Pulses. ACS Nano 17 (12), S. 11439-11453.

Veröffentlichungsdatum dieses Volltextes: 11 Mrz 2025 13:33
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.75215


Zusammenfassung

Photoluminescence from metal nanostructures following intense ultrashort illumination is a fundamental aspect of light–matter interactions. Surprisingly, many of its basic characteristics are under ongoing debate. Here, we resolve many of these debates by providing a comprehensive theoretical framework that describes this phenomenon and support it by an experimental confirmation. Specifically, we ...

Photoluminescence from metal nanostructures following intense ultrashort illumination is a fundamental aspect of light–matter interactions. Surprisingly, many of its basic characteristics are under ongoing debate. Here, we resolve many of these debates by providing a comprehensive theoretical framework that describes this phenomenon and support it by an experimental confirmation. Specifically, we identify aspects of the emission that are characteristic to either nonthermal or thermal emission, in particular, differences in the spectral and electric field dependence of these two contributions to the emission. Overall, nonthermal emission is characteristic of the early stages of light emission, while the later stages show thermal characteristics. The former dominate only for moderately high illumination intensities for which the electron temperature reached after thermalization remains close to room temperature.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftACS Nano
Verlag:American Chemical Society (ACS)
Band:17
Nummer des Zeitschriftenheftes oder des Kapitels:12
Seitenbereich:S. 11439-11453
Datum8 Juni 2023
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Lupton > Arbeitsgruppe John Lupton
Identifikationsnummer
WertTyp
10.1021/acsnano.3c01016DOI
Stichwörter / Keywordsplasmonics, electron nonequilibrium, photoluminescence, thermo-optic effects, metal nanoparticles
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
Dokumenten-ID75215

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