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Spin relaxation dynamics of radical-pair processes at low magnetic
fields
Tennahewa, T. H., Hosseinzadeh, S., Atwood, S. I., Popli, H., Malissa, H.
, Lupton, John M.
and Boehme, C.
(2022)
Spin relaxation dynamics of radical-pair processes at low magnetic
fields. arXiv.
Date of publication of this fulltext: 11 Mar 2025 14:05
Article
Abstract
We report measurements of room-temperature spin-relaxation times $T_1$ and $T_2$ of charge-carrier spins in a $\pi$-conjugated polymer thin film under bipolar injection and low ($1\mbox{ mT}\lesssim B_0\lesssim 10\mbox{ mT}$) static magnetic fields, using electrically detected magnetic resonant Hahn-echo and inversion-recovery pulse sequences. The experiments confirm the correlation between ...
We report measurements of room-temperature spin-relaxation times and
of charge-carrier spins in a
-conjugated polymer thin film under
bipolar injection and low ()
static magnetic fields, using electrically detected magnetic resonant Hahn-echo
and inversion-recovery pulse sequences. The experiments confirm the correlation
between the magnetic-field sensitive observables of radical-pair processes,
which include both the spin-dependent recombination currents in organic
semiconductors and the associated spin-relaxation times when random local
hyperfine fields and external magnetic fields compete in magnitude. Whereas a
striking field dependence of spin-lattice relaxation exists in the low-field
regime, the apparent spin decoherence time remains field independent as the
distinction between the two is lifted at low fields.
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Details
| Item type | Article | ||||||
| Journal or Publication Title | arXiv | ||||||
| Date | 14 July 2022 | ||||||
| Institutions | Physics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton | ||||||
| Projects |
Funded by:
Deutsche Forschungsgemeinschaft (DFG)
(314695032)
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| Identification Number |
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| Related URLs |
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| Dewey Decimal Classification | 500 Science > 530 Physics | ||||||
| Status | Published | ||||||
| Refereed | Unknown | ||||||
| Created at the University of Regensburg | Yes | ||||||
| URN of the UB Regensburg | urn:nbn:de:bvb:355-epub-752168 | ||||||
| Item ID | 75216 |
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