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Tennahewa, T. H. ; Hosseinzadeh, S. ; Atwood, S. I. ; Popli, H. ; Malissa, H. ; Lupton, John M. ; Boehme, C.

Spin relaxation dynamics of radical-pair processes at low magnetic
fields

Tennahewa, T. H., Hosseinzadeh, S., Atwood, S. I., Popli, H., Malissa, H. , Lupton, John M. and Boehme, C. (2022) Spin relaxation dynamics of radical-pair processes at low magnetic
fields.
arXiv.

Date of publication of this fulltext: 11 Mar 2025 14:05
Article


Abstract

We report measurements of room-temperature spin-relaxation times $T_1$ and $T_2$ of charge-carrier spins in a $\pi$-conjugated polymer thin film under bipolar injection and low ($1\mbox{ mT}\lesssim B_0\lesssim 10\mbox{ mT}$) static magnetic fields, using electrically detected magnetic resonant Hahn-echo and inversion-recovery pulse sequences. The experiments confirm the correlation between ...

We report measurements of room-temperature spin-relaxation times $T_1$ and
$T_2$ of charge-carrier spins in a $\pi$-conjugated polymer thin film under
bipolar injection and low ($1\mbox{ mT}\lesssim B_0\lesssim 10\mbox{ mT}$)
static magnetic fields, using electrically detected magnetic resonant Hahn-echo
and inversion-recovery pulse sequences. The experiments confirm the correlation
between the magnetic-field sensitive observables of radical-pair processes,
which include both the spin-dependent recombination currents in organic
semiconductors and the associated spin-relaxation times when random local
hyperfine fields and external magnetic fields compete in magnitude. Whereas a
striking field dependence of spin-lattice relaxation exists in the low-field
regime, the apparent spin decoherence time remains field independent as the
distinction between the two is lifted at low fields.



Involved Institutions


Details

Item typeArticle
Journal or Publication TitlearXiv
Date14 July 2022
InstitutionsPhysics > Institute of Experimental and Applied Physics > Chair Professor Lupton > Group John Lupton
Projects
Funded by: Deutsche Forschungsgemeinschaft (DFG) (314695032)
Identification Number
ValueType
2207.07086v1arXiv ID
10.1103/PhysRevB.109.075303DOI
Related URLs
URLURL Type
http://arxiv.org/abs/2207.07086v1Preprint
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedUnknown
Created at the University of RegensburgYes
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-752168
Item ID75216

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