Direkt zum Inhalt

Shao, Yiming ; Dirnberger, Florian ; Qui, Siyuan ; Acharya, Swagata ; Terres, Sophia ; Telford, Evan J. ; Pashov, Dimitar ; Kim, Brian S. Y. ; Ruta, Francesco L. ; Chica, Daniel G. ; Dismukes, Avalon H. ; Ziebel, Michael E. ; Wang, Yiping ; Choe, Jeongheon ; Bae, Youn Jue ; Millis, Andrew J. ; Katsnelson, Mikhail I. ; Mosina, Kseniia ; Sofer, Zdeněk ; Huber, Rupert ; Zhu, Xiaoyang ; Roy, Xavier ; van Schilfgaarde, Mark ; Chernikov, Alexey ; Basov, D. N.

Magnetically confined surface and bulk excitons in a layered antiferromagnet

Shao, Yiming, Dirnberger, Florian , Qui, Siyuan, Acharya, Swagata, Terres, Sophia, Telford, Evan J., Pashov, Dimitar, Kim, Brian S. Y., Ruta, Francesco L., Chica, Daniel G., Dismukes, Avalon H., Ziebel, Michael E., Wang, Yiping, Choe, Jeongheon, Bae, Youn Jue, Millis, Andrew J., Katsnelson, Mikhail I., Mosina, Kseniia, Sofer, Zdeněk, Huber, Rupert , Zhu, Xiaoyang, Roy, Xavier, van Schilfgaarde, Mark, Chernikov, Alexey und Basov, D. N. (2025) Magnetically confined surface and bulk excitons in a layered antiferromagnet. Nature Materials 24, S. 391-398.

Veröffentlichungsdatum dieses Volltextes: 02 Jul 2025 10:43
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.76925


Zusammenfassung

The discovery of two-dimensional van der Waals magnets has greatly expanded our ability to create and control nanoscale quantum phases. A unique capability emerges when a two-dimensional magnet is also a semiconductor that features tightly bound excitons with large oscillator strengths that fundamentally determine the optical response and are tunable with magnetic fields. Here we report a ...

The discovery of two-dimensional van der Waals magnets has greatly expanded our ability to create and control nanoscale quantum phases. A unique capability emerges when a two-dimensional magnet is also a semiconductor that features tightly bound excitons with large oscillator strengths that fundamentally determine the optical response and are tunable with magnetic fields. Here we report a previously unidentified type of optical excitation—a magnetic surface exciton—enabled by the antiferromagnetic spin correlations that confine excitons to the surface of CrSBr. Magnetic surface excitons exhibit stronger Coulomb attraction, leading to a higher binding energy than excitons confined in bulk layers, and profoundly alter the optical response of few-layer crystals. Distinct magnetic confinement of surface and bulk excitons is established by layer- and temperature-dependent exciton reflection spectroscopy and corroborated by ab initio many-body perturbation theory calculations. By quenching interlayer excitonic interactions, the antiferromagnetic order of CrSBr strictly confines the bound electron–hole pairs within the same layer, regardless of the total number of layers. Our work unveils unique confined excitons in a layered antiferromagnet, highlighting magnetic interactions as a vital approach for nanoscale quantum confinement, from few layers to the bulk limit.



Beteiligte Einrichtungen


Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftNature Materials
Verlag:Nature Publishing Group
Band:24
Seitenbereich:S. 391-398
Datum19 Februar 2025
InstitutionenPhysik > Institut für Experimentelle und Angewandte Physik > Lehrstuhl Professor Huber > Arbeitsgruppe Rupert Huber
Regensburg Center for Ultrafast Nanoscopy (RUN)
Projekte
Gefördert von: Deutsche Forschungsgemeinschaft (DFG) (314695032)
Identifikationsnummer
WertTyp
10.1038/s41563-025-02129-6DOI
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
Dokumenten-ID76925

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