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Nonequilibrium resonant spectroscopy of molecular vibrons
Ryndyk, Dmitry und Cuniberti, Gianaurelio
(2007)
Nonequilibrium resonant spectroscopy of molecular vibrons.
Physical Review B 76, S. 155430.
Veröffentlichungsdatum dieses Volltextes: 05 Aug 2009 13:57
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.7794
Zusammenfassung
Quantum transport through single molecules is essentially affected by molecular vibrations. We investigate the behavior of the prototype single-level model with weak to intermediate electron-vibron interactions and arbitrary couplings to the leads. For this, we have developed a nonequilibrium self-consistent theory which allows us to explore the nonperturbative regime via the nonequilibrium Green ...
Quantum transport through single molecules is essentially affected by molecular vibrations. We investigate the behavior of the prototype single-level model with weak to intermediate electron-vibron interactions and arbitrary couplings to the leads. For this, we have developed a nonequilibrium self-consistent theory which allows us to explore the nonperturbative regime via the nonequilibrium Green function formalism. We show that the nonequilibrium resonant spectroscopy is able to determine the energies of molecular orbitals and the spectrum of molecular vibrations. Our results are relevant to scanning tunneling spectroscopy experiments and demonstrate the importance of the systematic and self-consistent investigation of the effects of the vibronic dynamics onto the transport through single molecules.
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| Dokumentenart | Artikel | ||||
| Titel eines Journals oder einer Zeitschrift | Physical Review B | ||||
| Verlag: | AMER PHYSICAL SOC | ||||
|---|---|---|---|---|---|
| Ort der Veröffentlichung: | COLLEGE PK | ||||
| Band: | 76 | ||||
| Seitenbereich: | S. 155430 | ||||
| Datum | 2007 | ||||
| Institutionen | Physik > Institut für Theoretische Physik > Entpflichtete oder im Ruhestand befindliche Professoren > Arbeitsgruppe Gianaurelio Cuniberti Physik > Institut für Theoretische Physik > Lehrstuhl Professor Richter > Arbeitsgruppe Klaus Richter | ||||
| Identifikationsnummer |
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| Stichwörter / Keywords | SCANNING-TUNNELING-MICROSCOPY; ELECTRON-PHONON INTERACTION; JUNCTIONS; ADSORBATES; TRANSPORT; NANOSTRUCTURES; CONDUCTANCE; TRANSISTORS; MODEL; FIELD; | ||||
| Dewey-Dezimal-Klassifikation | 500 Naturwissenschaften und Mathematik > 530 Physik | ||||
| Status | Veröffentlicht | ||||
| Begutachtet | Ja, diese Version wurde begutachtet | ||||
| An der Universität Regensburg entstanden | Ja | ||||
| URN der UB Regensburg | urn:nbn:de:bvb:355-epub-77942 | ||||
| Dokumenten-ID | 7794 |
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