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Zollner, Klaus ; Cvitkovich, Lukas ; Silvioli, Riccardo ; Stier, Andreas V. ; Fabian, Jaroslav

Resonant magnetic proximity hot spots in Co/hBN/graphene

Article

Zollner, Klaus , Cvitkovich, Lukas , Silvioli, Riccardo , Stier, Andreas V. and Fabian, Jaroslav (2026) Resonant magnetic proximity hot spots in Co/hBN/graphene. Physical Review B 113, p. 235142.

DOI to cite this document: 10.5283/epub.79729

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Abstract

Magnetic proximity effects in Co/hBN/graphene heterostructures are systematically analyzed via first-principles calculations, demonstrating a pronounced localized spatial variation of the induced spin polarization of graphene's Dirac states. The proximity-induced exchange coupling, magnetic moments, and tunneling spin polarization (TSP) are shown to depend sensitively on the atomic registry at ...

Magnetic proximity effects in Co/hBN/graphene heterostructures are systematically analyzed via first-principles calculations, demonstrating a pronounced localized spatial variation of the induced spin polarization of graphene's Dirac states. The proximity-induced exchange coupling, magnetic moments, and tunneling spin polarization (TSP) are shown to depend sensitively on the atomic registry at the interfaces. We analyze more than 20 distinct stackings—including high- and low-symmetry configurations—and reveal that the spin splittings of graphene's Dirac bands span a wide range from 1 to 100 meV, depending on the local hybridization of Co dz2, hBN pz, and graphene pz orbitals. The strongest proximity effects emerge at geometric resonances, or “proximity hot spots”, where the three orbital states overlap maximally. The local spin polarization also depends sensitively on energy: Dirac states aligned with resonant Co orbitals experience the most pronounced exchange interaction. At these energies, the pseudospin Hamiltonian description of magnetic proximity effects breaks down. Outside these resonances, the pseudospin picture is restored. Our findings highlight the intrinsically local nature of proximity effects, governed by the spectral resonance and interlayer wave function overlap. We further quantify how additional hBN layers, interlayer twist, and multilayer graphene modify the proximity exchange and TSP, offering microscopic insight for designing spintronic van der Waals heterostructures with engineered interfaces and optimized spin transport.



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Details

Item typeArticle
Journal or Publication TitlePhysical Review B
PublisherAmerican Physical Society (APS)
Volume113
Page Rangep. 235142
Date23 June 2026
Date of publication01 Jul 2026 07:00
InstitutionsPhysics > Halle-Berlin-Regensburg Cluster of Excellence CCE
Physics > Institute of Theroretical Physics > Chair Professor Richter > Group Jaroslav Fabian
Projects
Funded by: Deutsche Forschungsgemeinschaft (DFG) (314695032)
Funded by: Deutsche Forschungsgemeinschaft (DFG) (422707584)
Identification Number
ValueType
10.1103/f1l3-xqzxDOI
Keywordsfirst-principles calculations, magnetic proximity effect, van der Waals materials
Dewey Decimal Classification500 Science > 530 Physics
StatusPublished
RefereedYes, this version has been refereed
Created at the University of RegensburgPartially
URN of the UB Regensburgurn:nbn:de:bvb:355-epub-797297
Item ID79729

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