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Zollner, Klaus ; Cvitkovich, Lukas ; Silvioli, Riccardo ; Stier, Andreas V. ; Fabian, Jaroslav

Resonant magnetic proximity hot spots in Co/hBN/graphene

Zollner, Klaus , Cvitkovich, Lukas , Silvioli, Riccardo , Stier, Andreas V. und Fabian, Jaroslav (2026) Resonant magnetic proximity hot spots in Co/hBN/graphene. Physical Review B 113, S. 235142.

Veröffentlichungsdatum dieses Volltextes: 01 Jul 2026 07:00
Artikel
DOI zum Zitieren dieses Dokuments: 10.5283/epub.79729

Dies ist die aktuelle Version dieses Eintrags.


Zusammenfassung

Magnetic proximity effects in Co/hBN/graphene heterostructures are systematically analyzed via first-principles calculations, demonstrating a pronounced localized spatial variation of the induced spin polarization of graphene's Dirac states. The proximity-induced exchange coupling, magnetic moments, and tunneling spin polarization (TSP) are shown to depend sensitively on the atomic registry at ...

Magnetic proximity effects in Co/hBN/graphene heterostructures are systematically analyzed via first-principles calculations, demonstrating a pronounced localized spatial variation of the induced spin polarization of graphene's Dirac states. The proximity-induced exchange coupling, magnetic moments, and tunneling spin polarization (TSP) are shown to depend sensitively on the atomic registry at the interfaces. We analyze more than 20 distinct stackings—including high- and low-symmetry configurations—and reveal that the spin splittings of graphene's Dirac bands span a wide range from 1 to 100 meV, depending on the local hybridization of Co dz2, hBN pz, and graphene pz orbitals. The strongest proximity effects emerge at geometric resonances, or “proximity hot spots”, where the three orbital states overlap maximally. The local spin polarization also depends sensitively on energy: Dirac states aligned with resonant Co orbitals experience the most pronounced exchange interaction. At these energies, the pseudospin Hamiltonian description of magnetic proximity effects breaks down. Outside these resonances, the pseudospin picture is restored. Our findings highlight the intrinsically local nature of proximity effects, governed by the spectral resonance and interlayer wave function overlap. We further quantify how additional hBN layers, interlayer twist, and multilayer graphene modify the proximity exchange and TSP, offering microscopic insight for designing spintronic van der Waals heterostructures with engineered interfaces and optimized spin transport.



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Details

DokumentenartArtikel
Titel eines Journals oder einer ZeitschriftPhysical Review B
Verlag:American Physical Society (APS)
Band:113
Seitenbereich:S. 235142
Datum23 Juni 2026
InstitutionenPhysik > Halle-Berlin-Regensburg Cluster of Excellence CCE
Physik > Institut für Theoretische Physik > Lehrstuhl Professor Richter > Arbeitsgruppe Jaroslav Fabian
Projekte
Gefördert von: Deutsche Forschungsgemeinschaft (DFG) (314695032)
Gefördert von: Deutsche Forschungsgemeinschaft (DFG) (422707584)
Identifikationsnummer
WertTyp
10.1103/f1l3-xqzxDOI
Stichwörter / Keywordsfirst-principles calculations, magnetic proximity effect, van der Waals materials
Dewey-Dezimal-Klassifikation500 Naturwissenschaften und Mathematik > 530 Physik
StatusVeröffentlicht
BegutachtetJa, diese Version wurde begutachtet
An der Universität Regensburg entstandenZum Teil
URN der UB Regensburgurn:nbn:de:bvb:355-epub-797297
Dokumenten-ID79729

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