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Diffusion in ionic liquids: the interplay between molecular structure and dynamics

Sangoro, Joshua and Iacob, Ciprian and Naumov, S. and Valiullin, R. and Rexhausen, H. and Hunger, J. and Buchner, Richard and Strehmel, V. and Kärger, J. and Kremer, Friedrich (2011) Diffusion in ionic liquids: the interplay between molecular structure and dynamics. Soft Matter 7 (5), pp. 1678-1681.

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Abstract

Diffusion in a series of ionic liqs. is investigated by a combination of Broadband Dielec. Spectroscopy (BDS) and Pulsed Field Gradient NMR (PFG NMR). It is demonstrated that the mean jump lengths increase with the mol. vols. detd. from quantum-chem. calcns. This provides a direct means-via Einstein-Smoluchowski relation-to det. the diffusion coeff. by BDS over more than 8 decades unambiguously ...

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Item Type:Article
Date:2011
Institutions:Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry VI - Physical Chemistry (Solution Chemistry) > PD Dr. Richard Buchner
Identification Number:
ValueType
10.1039/c0sm01404dDOI
Keywords:ionic liq diffusion mol structure dynamics
Subjects:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Owner: Georg Berger
Deposited On:06 Jun 2012 13:55
Last Modified:06 Jun 2012 13:55
Item ID:24713
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