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Influence of Concentration and Temperature on the Dynamics of Water in the Hydrophobic Hydration Shell of Tetramethylurea

Tielrooij, K.-J. and Hunger, J. and Hefter, Glenn and Buchner, Richard and Bonn, M. and Bakker, H.J. (2010) Influence of Concentration and Temperature on the Dynamics of Water in the Hydrophobic Hydration Shell of Tetramethylurea. Journal of the American Chemical Society 132 (44), pp. 15671-15678.

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Abstract

We study the influence of the amphipilic compd. tetramethylurea (TMU) on the dynamical properties of water, using dielec. relaxation spectroscopy in the regime between 0.2 GHz and 2 THz. This technique is capable of resolving different water species, their relative fractions, and their corresponding reorientation dynamics. We find that the reorientation dynamics of water mols. in the hydration ...

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Item Type:Article
Date:2010
Institutions:Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry VI - Physical Chemistry (Solution Chemistry) > PD Dr. Richard Buchner
Identification Number:
ValueType
10.1021/ja106273wDOI
Keywords:dynamics water hydrophobic hydration shell tetramethylurea dielec relaxation
Subjects:500 Science > 540 Chemistry & allied sciences
Status:Published
Refereed:Yes, this version has been refereed
Created at the University of Regensburg:Yes
Owner: Georg Berger
Deposited On:06 Jun 2012 13:48
Last Modified:06 Jun 2012 13:48
Item ID:24721
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