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Importance of initial and final states as intermediate states in two-photon spectroscopy of polar molecules

Dick, Bernhard and Hohlneicher, Georg (1982) Importance of initial and final states as intermediate states in two-photon spectroscopy of polar molecules. Journal of Chemical Physics 76 (12), pp. 5755-5760.

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Abstract

Two-photon transitions may proceed via a mechanism not involving virtually excited intermediate states. This mechanism may account for the largest contribution to the 2-photon cross section in polar mols. if the dipole moment strongly alters with excitation. Possible consequences for the 2-photon detection of forbidden states in polar polyene systems are discussed.

Item Type:

Article

Additional information (public):

CAN 97:100809 73-1 Optical, Electron, and Mass Spectroscopy and Other Related Properties

Institutions:

Chemistry and Pharmacy > Institut für Physikalische und Theoretische Chemie > Chair of Chemistry III - Physical Chemistry (Light and Matter) > Prof. Dr. Bernhard Dick

Identification Number:

Value	Type
1982:500809	Other
10.1063/1.442971	DOI

Keywords:

Energy level (forbidden, in polar polyene systems, 2-photon transition in relation to); Photon (transition of 2, in polar mols.); Energy level transition (two-photon, of polar mols., mechanism of); two photon transition polar mol

Subjects:

500 Science > 540 Chemistry & allied sciences

Status:

Published

Refereed:

Yes, this version has been refereed

Created at the University of Regensburg:

Owner:

Prof. Dr. Bernhard Dick

Deposited On:

22 Jan 2009 11:27

Last Modified: