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Organocuprate Conjugate Addition: The Structural Features of Diastereomeric and Supramolecular p-Intermediates

Henze, W. ; Gärtner, T. ; Gschwind, R. M.


In the reaction pathway of conjugate additions with organocuprate reagents, Cu(I) π-complexes and Cu(III) σ-complexes have been identified as central, NMR-detectable intermediate species. However, no experimental evidence for the structures of π-intermediates with extensive chiral enones or the principal aggregation level and aggregate structure of π-complexes in diethyl ether has been available ...


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