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Electronic Structure and Spectroscopic Properties of Copper Catecholate Complexes with Interligand Charge Transfer Behavior

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Benedix, R. ; Vogler, Arnd
Date of publication of this fulltext: 17 Mar 2010 09:03


The structural and spectroscopic properties of copper catecholate complexes with nitrogen ligands of the α- diimine type are studied by qualitative MO considerations. The characteristic feature of these donor acceptor systems is an interligand charge-transfer from the catecholate donor to the α-diimine acceptor site. The dependence of the interligand charge-transfer absorption band on the energies of the acceptor and the donor levels as well as on the solvent polarity is discussed.

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