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Vibronic and magnetic coupling in the radiative deactivation of the lowest excited states of [Os(bpy)₃]²⁺ doped into [Ru(bpy)₃](PF₆)₂

Braun, D. ; Hensler, G. ; Gallhuber, E. ; Yersin, Hartmut



Abstract

Small amounts of [Os(bpy)₃]²⁺+ doped into single-crystal [Ru(bpy)₃](PF₆)₂ exhibit highly resolved MLCT spectra corresponding to the transitions between the ground state and the lowest excited states. The electronic origin as well as the vibronic satellites appear as sharp lines with half-widths of ca. 2 cm⁻¹. Three distinct spectroscopic sites are identified. For the lowest energy site the lowest ...

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