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Geometrical distortions in excited A₂' states of single-crystal [Ru(bpy)₃](PF₆)₂

Schönherr, T. ; Degen, J. ; Gallhuber, E. ; Hensler, G. ; Yersin, Hartmut


The absorption band pattern of the E || c-polarized metal-to-ligand charge-transfer transitions in [Ru(bpy)₃](PF₆)₂ have been investigated by a band profile analysis in terms of intensity distributions l(η; Δ, β) of vibrational progressions in totally symmetric normal modes. For a specific state at 18770 cm⁻¹ of A₂' symmetry (classified in the relevant double group D₃') the Δ parameter obtained ...


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